Unravelling the dynamical origin of below- and near-threshold harmonic generation of H2+ in an intense NIR laser field
dc.contributor.author | Heslar, John | |
dc.contributor.author | Chu, Shih-I | |
dc.date.accessioned | 2016-12-16T21:42:33Z | |
dc.date.available | 2016-12-16T21:42:33Z | |
dc.date.issued | 2016-11-24 | |
dc.identifier.citation | Heslar, John, and Shih-I. Chu. "Unravelling the Dynamical Origin of Below- and Near-threshold Harmonic Generation of H2 in an Intense NIR Laser Field." Scientific Reports 6 (2016): 37774. | en_US |
dc.identifier.uri | http://hdl.handle.net/1808/22256 | |
dc.description.abstract | Recently, the study of near- and below- threshold regime harmonics as a potential source of intense coherent vacuum-ultraviolet radiation has received considerable attention. However, the dynamical origin of these lower harmonics, particularly for the molecular systems, is less understood and largely unexplored. Here we perform the first fully ab initio and high precision 3D quantum study of the below- and near-threshold harmonic generation of molecules in an intense 800-nm near-infrared (NIR) laser field. Combining with a synchrosqueezing transform of the quantum time-frequency spectrum and an extended semiclassical analysis, we explore in-depth the roles of various quantum trajectories, including short- and long trajectories, multiphoton trajectories, resonance-enhanced trajectories, and multiple rescattering trajectories of the below- and near- threshold harmonic generation processes. Our results shed new light on the dynamical origin of the below- and near-threshold harmonic generation and various quantum trajectories for diatomic molecules for the first time. | en_US |
dc.publisher | Nature Publishing Group | en_US |
dc.relation.isversionof | http://www.nature.com/articles/srep37774 | en_US |
dc.rights | This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ | en_US |
dc.rights.uri | http://creativecommons.org/licenses/by/4.0/ | |
dc.subject | Atomic and molecular interactions with photons | en_US |
dc.subject | High-harmonic generation | en_US |
dc.title | Unravelling the dynamical origin of below- and near-threshold harmonic generation of H2+ in an intense NIR laser field | en_US |
dc.type | Article | en_US |
kusw.kuauthor | Chu, Shih-I | |
kusw.kudepartment | Chemistry | en_US |
dc.identifier.doi | 10.1038/srep37774 | en_US |
kusw.oaversion | Scholarly/refereed, publisher version | en_US |
kusw.oapolicy | This item meets KU Open Access policy criteria. | en_US |
dc.rights.accessrights | openAccess |
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Except where otherwise noted, this item's license is described as: This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/