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Mixed-conducting oxygen permeable ceramic membranes for the carbon dioxide reforming of methane
dc.contributor.author | Slade, David A. | |
dc.contributor.author | Duncan, Andrew M. | |
dc.contributor.author | Nordheden, Karen J. | |
dc.contributor.author | Williams, Susan Michelle | |
dc.date.accessioned | 2015-11-16T16:26:20Z | |
dc.date.available | 2015-11-16T16:26:20Z | |
dc.date.issued | 2007-02-01 | |
dc.identifier.citation | Slade, David A., Andrew M. Duncan, Karen J. Nordheden, and Susan M. Stagg-Williams. "Mixed-conducting Oxygen Permeable Ceramic Membranes for the Carbon Dioxide Reforming of Methane." Green Chemistry Green Chem. 9.6 (2007): 577. http://dx.doi.org/10.1039/B614232J | en_US |
dc.identifier.uri | http://hdl.handle.net/1808/18920 | |
dc.description | This is the published version. Copyright 2007 Royal Society of Chemistry | en_US |
dc.description.abstract | Due to the high economic, environmental, and safety costs associated with pure oxygen, mixed-conducting oxygen-permeable ceramic membranes are being explored as an alternative oxygen source for hydrocarbon conversion reactors. This work reports a dramatic improvement in catalyst performance when an oxygen-permeable SrFeCo0.5Ox ceramic membrane is used in conjunction with a conventional powder Pt/ZrO2 catalyst for the CO2 reforming of CH4. Experiments comparing catalyst performance with up to 2% co-fed oxygen to catalyst performance with oxygen from the ceramic membrane demonstrated a conversion three times higher with the membrane than with any amount of co-fed oxygen. The results suggest that membrane oxygen is more beneficial for catalyst activity and stability than molecular gas-phase oxygen. | en_US |
dc.publisher | Royal Society of Chemistry | en_US |
dc.title | Mixed-conducting oxygen permeable ceramic membranes for the carbon dioxide reforming of methane | en_US |
dc.type | Article | |
kusw.kuauthor | Nordheden, Karen J. | |
kusw.kuauthor | Williams, Susan Michelle | |
kusw.kudepartment | Chemical & Petroleum Engr | en_US |
dc.identifier.doi | 10.1039/B614232J | |
kusw.oaversion | Scholarly/refereed, publisher version | |
kusw.oapolicy | This item does not meet KU Open Access policy criteria. | |
dc.rights.accessrights | openAccess |