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    Exploration of Coulomb explosion dynamics through excited vibrational states of molecules

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    Issue Date
    2005-01-31
    Author
    Zhou, Zhongyuan
    Chu, Shih-I
    Publisher
    American Physical Society
    Type
    Article
    Article Version
    Scholarly/refereed, publisher version
    Metadata
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    Abstract
    The fragmentation dynamics of H2+ molecular ions in intense laser fields is investigated by means of a high-precision ab initio method beyond the Born-Oppenheimer approximation. Special attention is paid to the detailed Coulomb explosion (CE) mechanisms and dynamics through excited vibrational states of H2+. A kinetic-energy release (KER) spectrum and CE phenomenon is predicted, in which the kinetic-energy distribution of H+ ions exhibits a series of peaks separated by one photon energy. A proposed scheme for observation of the KER spectrum and CE dynamics is presented.
    URI
    http://hdl.handle.net/1808/16039
    DOI
    https://doi.org/10.1103/PhysRevA.71.011402
    Collections
    • Chemistry Scholarly Works [610]
    Citation
    Zhou, Zhongyuan and Chu, Shih-I. "Exploration of Coulomb explosion dynamics through excited vibrational states of molecules." Phys. Rev. A 71, 011402(R) – Published 31 January 2005 http://dx.doi.org/10.1103/PhysRevA.71.011402

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    Contact KU ScholarWorks
    785-864-8983
    KU Libraries
    1425 Jayhawk Blvd
    Lawrence, KS 66045
    785-864-8983

    KU Libraries
    1425 Jayhawk Blvd
    Lawrence, KS 66045
    Image Credits
     

     

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