KUKU

KU ScholarWorks

  • myKU
  • Email
  • Enroll & Pay
  • KU Directory
    • Login
    View Item 
    •   KU ScholarWorks
    • Geography & Atmospheric Science
    • Geography & Atmospheric Science Scholarly Works
    • View Item
    •   KU ScholarWorks
    • Geography & Atmospheric Science
    • Geography & Atmospheric Science Scholarly Works
    • View Item
    JavaScript is disabled for your browser. Some features of this site may not work without it.

    Predicted change in global secondary organic aerosol concentrations in response to future climate, emissions, and land use change

    Thumbnail
    View/Open
    Feddema_Secondary_Organic_Aerosol_Concentrations.pdf (1.383Mb)
    Issue Date
    2008-03
    Author
    Heald, C. L.
    Henze, D. K.
    Horowitz, L. W.
    Feddema, Johannes J.
    Lamarque, J. F.
    Guenther, A.
    Hess, P. G.
    Vitt, F.
    Seinfeld, J. H.
    Goldstein, A. H.
    Fung, I.
    Publisher
    American Geophysical Union
    Type
    Article
    Article Version
    Scholarly/refereed, publisher version
    Metadata
    Show full item record
    Abstract
    The sensitivity of secondary organic aerosol (SOA) concentration to changes in climate and emissions is investigated using a coupled global atmosphere-land model driven by the year 2100 IPCC A1B scenario predictions. The Community Atmosphere Model (CAM3) is updated with recent laboratory determined yields for SOA formation from monoterpene oxidation, isoprene photooxidation and aromatic photooxidation. Biogenic emissions of isoprene and monoterpenes are simulated interactively using the Model of Emissions of Gases and Aerosols (MEGAN2) within the Community Land Model (CLM3). The global mean SOA burden is predicted to increase by 36% in 2100, primarily the result of rising biogenic and anthropogenic emissions which independently increase the burden by 26% and 7%. The later includes enhanced biogenic SOA formation due to increased emissions of primary organic aerosol (5–25% increases in surface SOA concentrations in 2100). Climate change alone (via temperature, removal rates, and oxidative capacity) does not change the global mean SOA production, but the global burden increases by 6%. The global burden of anthropogenic SOA experiences proportionally more growth than biogenic SOA in 2100 from the net effect of climate and emissions (67% increase predicted). Projected anthropogenic land use change for 2100 (A2) is predicted to reduce the global SOA burden by 14%, largely the result of cropland expansion. South America is the largest global source region for SOA in the present day and 2100, but Asia experiences the largest relative growth in SOA production by 2100 because of the large predicted increases in Asian anthropogenic aromatic emissions. The projected decrease in global sulfur emissions implies that SOA will contribute a progressively larger fraction of the global aerosol burden.
    Description
    Copyright 2008 by the American Geophysical Union. 0148-0227/08/2007JD009092
    URI
    http://hdl.handle.net/1808/9306
    DOI
    https://doi.org/10.1029/2007JD009092
    Collections
    • Geography & Atmospheric Science Scholarly Works [170]
    Citation
    Heald, C. L., et al. (2008), Predicted change in global secondary organic aerosol concentrations in response to future climate, emissions, and land use change, J. Geophys. Res., 113, D05211, http://dx.doi.org/10.1029/2007JD009092

    Items in KU ScholarWorks are protected by copyright, with all rights reserved, unless otherwise indicated.


    We want to hear from you! Please share your stories about how Open Access to this item benefits YOU.


    Contact KU ScholarWorks
    785-864-8983
    KU Libraries
    1425 Jayhawk Blvd
    Lawrence, KS 66045
    785-864-8983

    KU Libraries
    1425 Jayhawk Blvd
    Lawrence, KS 66045
    Image Credits
     

     

    Browse

    All of KU ScholarWorksCommunities & CollectionsThis Collection

    My Account

    LoginRegister

    Statistics

    View Usage Statistics

    Contact KU ScholarWorks
    785-864-8983
    KU Libraries
    1425 Jayhawk Blvd
    Lawrence, KS 66045
    785-864-8983

    KU Libraries
    1425 Jayhawk Blvd
    Lawrence, KS 66045
    Image Credits
     

     

    The University of Kansas
      Contact KU ScholarWorks
    Lawrence, KS | Maps
     
    • Academics
    • Admission
    • Alumni
    • Athletics
    • Campuses
    • Giving
    • Jobs

    The University of Kansas prohibits discrimination on the basis of race, color, ethnicity, religion, sex, national origin, age, ancestry, disability, status as a veteran, sexual orientation, marital status, parental status, gender identity, gender expression and genetic information in the University’s programs and activities. The following person has been designated to handle inquiries regarding the non-discrimination policies: Director of the Office of Institutional Opportunity and Access, IOA@ku.edu, 1246 W. Campus Road, Room 153A, Lawrence, KS, 66045, (785)864-6414, 711 TTY.

     Contact KU
    Lawrence, KS | Maps