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Annulation of Perimidines with 5-Alkynylpyrimidines en Route to 7-Formyl-1,3-Diazopyrenes
Shcherbakov, Stanislav V. Aksenov, Alexander V. Vendin, Maksim V. Shcherbakova, Viktoria Yu. Ivanova, Anna Yu. Shcheglov, Maksim O. Ovcharov, Sergei N. Rubin, Michael
Shcherbakov, Stanislav V.
Aksenov, Alexander V.
Vendin, Maksim V.
Shcherbakova, Viktoria Yu.
Ivanova, Anna Yu.
Shcheglov, Maksim O.
Ovcharov, Sergei N.
Rubin, Michael
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Abstract
Unusual rearrangements were shown to accompany Brønsted acid-assisted peri-annulations of 1H-perimidines with 5-alkynylpyrimidines. These transformations take different routes depending on the nature of acetylene precursor, and lead to the formation of 7-formyl-1,3-diazopyrenes.
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2022-12-10
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MDPI
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Shcherbakov_2022.pdf
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Annulations, Acetylenes, Nitrogen heterocycles, Brønsted acid catalysis, Rearrangements
Citation
Shcherbakov, S.V.; Aksenov, A.V.; Vendin, M.V.; Shcherbakova, V.Y.; Ivanova, A.Y.; Shcheglov, M.O.; Ovcharov, S.N.; Rubin, M. Annulation of Perimidines with 5-Alkynylpyrimidines en Route to 7-Formyl-1,3-Diazopyrenes. Int. J. Mol. Sci. 2022, 23, 15657. https://doi.org/10.3390/ijms232415657