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Synthesis and Applications of Amide-Based Pd(II) NNN-pincer Complexes
Johnson, Thomas Seals
Johnson, Thomas Seals
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Abstract
The first project is described in Chapter 2, and details the synthesis of a series of mono- and multimetallic Pd(II) NNN-pincer complexes which—to the best of our knowledge—represent the first examples of these types of complexes being employed as catalysts in a Heck reaction. Chapter 3 discusses the design and synthesis of a hybrid pincer/imidazolium salt ligand and its transition metal chemistry, with the ultimate goal of synthesizing heterobimetallic complexes for bifunctional catalysis. The work in Chapter 4 strays away from the catalysis theme, and includes preliminary investigations into the synthesis of metal-organic frameworks (MOF) derived from the combination of a bis[palladium(II)] complex with a pyridine-appended ditopic macrocycle.
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Date
2016-05-31
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University of Kansas
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Keywords
Chemistry, Inorganic chemistry, Organic chemistry, Catalysis, Heck Reaction, Heterobimetallic, Macrocycle, Palladium, Pincer