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Transformational dynamics of BZO and BHO nanorods imposed by Y2O3 nanoparticles for improved isotropic pinning in YBa2Cu3O7−δ thin films
Gautam, Bibek ; Sebastian, Mary Ann ; Chen, Shihong ; Shi, Jack J. ; Haugan, Timothy ; Xing, Zhongwen ; Zhang, Wenrui ; Huang, Jijie ; Wang, Haiyan ; Osofsky, Mike ... show 2 more
Gautam, Bibek
Sebastian, Mary Ann
Chen, Shihong
Shi, Jack J.
Haugan, Timothy
Xing, Zhongwen
Zhang, Wenrui
Huang, Jijie
Wang, Haiyan
Osofsky, Mike
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Abstract
An elastic strain model was applied to evaluate the rigidity of the c-axis aligned one-dimensional artificial pinning centers (1D-APCs) in YBa2Cu3O7-δ matrix films. Higher rigidity was predicted for BaZrO3 1D-APCs than that of the BaHfO3 1D-APCs. This suggests a secondary APC doping of Y2O3 in the 1D-APC/YBa2Cu3O7-δ nanocomposite films would generate a stronger perturbation to the c-axis alignment of the BaHfO3 1D-APCs and therefore a more isotropic magnetic vortex pinning landscape. In order to experimentally confirm this, we have made a comparative study of the critical current density Jc (H, θ, T) of 2 vol.% BaZrO3 + 3 vol.%Y2O3 and 2 vol.%BaHfO3 + 3 vol.%Y2O3 double-doped (DD) YBa2Cu3O7-δ films deposited at their optimal growth conditions. A much enhanced isotropic pinning was observed in the BaHfO3 DD samples. For example, at 65 K and 9.0 T, the variation of the Jc across the entire θ range from θ=0 (H//c) to θ=90 degree (H//ab) is less than 18% for BaHfO3 DD films, in contrast to about 100% for the BaZrO3 DD counterpart. In addition, lower α values from the Jc(H) ∼ H-α fitting were observed in the BaHfO3 DD films in a large θ range away from the H//c-axis. Since the two samples have comparable Jc values at H//c-axis, the improved isotropic pinning in BaHfO3 DD films confirms the theoretically predicted higher tunability of the BaHfO3 1D-APCs in APC/YBa2Cu3O7-δ nanocomposite films.
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2017
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AIP Publishing
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Gautam, B., Sebastian, M. A., Chen, S., Shi, J., Haugan, T., Xing, Z., ... & Prestigiacomo, J. (2017). Transformational dynamics of BZO and BHO nanorods imposed by Y2O3 nanoparticles for improved isotropic pinning in YBa2Cu3 O 7-δ thin films. AIP Advances, 7(7), 075308.
